Transmutations of Long-Lived and Medium-Lived Fission Products Extracted from CANDU and PWR Spent Fuels in an Accelerator-Driven System

Table 1

Atomic densities of isotopes used in the modified ADS (atoms/(barn·cm)).

Isotopes	Case A		Case B		Case C
	BOC	EOC	BOC	EOC	BOC	EOC
He^a	8.46569E − 03
Cr^b	3.66345E − 06
Fe	7.69324E − 06
Zr	3.59861E − 03
Sn	5.31202E − 05
Hf	3.66345E − 06
^16O^c	2.93697E − 02	1.02789E − 02	2.73042E − 02	9.55563E − 03	2.73680E − 02	9.57800E − 03
^232Th	—	1.00083E − 09	9.33110E − 12	9.33187E − 10	6.19031E − 03	1.85725E − 03
^233Pa	—	1.99410E − 11	—	2.24895E − 11	—	2.18856E − 06
^232U	—	1.48743E − 09	—	1.15799E − 09	—	7.29463E − 08
^233U	—	1.49174E − 09	—	1.73848E − 09	2.66993E − 05	1.71951E − 04
^234U	6.33080E − 07	1.73443E − 07	6.11203E − 08	1.27383E − 07	6.87464E − 07	1.43121E − 05
^235U	5.56078E − 05	7.42546E − 06	2.46375E − 04	4.42845E − 05	8.70822E − 05	1.29798E − 05
^236U	7.40277E − 06	4.58373E − 06	7.30603E − 05	3.06038E − 05	4.17128E − 05	1.52204E − 05
^238U	1.45193E − 02	4.34139E − 03	1.26922E − 02	3.82895E − 03	6.32613E − 03	1.81887E − 03
^235Np		3.60106E − 13	—	9.11276E − 12	—	1.73780E − 12
^236Np		2.59177E − 11	2.43482E − 11	1.97672E − 11	3.34642E − 12	3.10285E − 12
^237Np	2.12823E − 07	8.49462E − 07	6.13307E − 06	5.79906E − 06	3.20538E − 06	3.44686E − 06
^236Pu		4.56934E − 12	—	1.82719E − 11	—	1.46943E − 11
^237Pu		1.01802E − 11	—	1.19406E − 11	—	5.84736E − 12
^238Pu	1.71122E − 08	1.19518E − 06	2.00245E − 06	3.22821E − 06	1.23440E − 06	2.74465E − 06
^239Pu	2.82080E − 05	3.52240E − 04	9.21538E − 05	4.00820E − 04	3.10560E − 05	1.86319E − 04
^240Pu	7.09409E − 06	6.39388E − 05	3.01341E − 05	5.42331E − 05	2.05142E − 05	3.84026E − 05
^241Pu	1.02146E − 06	3.23992E − 05	1.63268E − 05	2.28933E − 05	6.20598E − 06	1.60207E − 05
^242Pu	1.58382E − 07	7.33230E − 06	4.50249E − 06	4.09549E − 06	3.81657E − 06	5.08140E − 06
^244Pu	—	9.79453E − 11	—	7.07767E − 11	2.26821E − 11	1.38317E − 10
^241Am	—	3.79692E − 06	—	3.62364E − 06	7.47539E − 07	3.26888E − 06
^243Am	—	1.29639E − 06	—	9.88034E − 07	1.92135E − 07	1.47667E − 06
^242Cm	—	2.77117E − 07	—	1.78654E − 07	1.18948E − 09	1.76447E − 07
^244Cm	—	3.61448E − 07	—	3.30190E − 07	1.33784E − 08	5.93151E − 07
^245Cm	—	1.45861E − 08		2.61196E − 08	1.50500E − 10	4.43606E − 08
^246Cm	—	2.26875E − 09	—	1.67286E − 09	4.11277E − 12	8.08843E − 09
^247Cm	—	3.13581E − 11	—	3.40359E − 11	—	2.00524E − 10
^248Cm	—	1.68813E − 12	—	1.43607E − 12	—	1.52560E − 11
^206Pb^d	3.56020E − 3
^207Pb	3.39702E − 3
^208Pb	7.87694E − 3
^209Bi	1.55345E − 2
^12C^e	1.05402E − 1

^aCoolant; ^bclad; ^cfuel; ^dtarget; ^ereflector.